What word (plural) best describes the four themed answers (what are they all famous as)? Then think of a 2-letter abbreviation for their common nationality, and put that before the other word.
In some puzzles, notably the Listener, the
only way to construct the square is with letter pairs from answers and the letters you have in the grid. No hint to the keyword can be given (this is in the Notes for Setters). Fortunately Azed spares us the pointless, mind-numbing tedium of doing this and usually gives a generous hint to the keyword, as here.