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Two 6-letter answers I'm not sure of. Firstly,
25 Down - "Cushion, with pins removed, spins over and over."
(S-F-E-) SOFTEN, I should imagine.
37 Across - "Substance initially becoming nitrogen gas." (N-T-E-)

37a natter - matter (substance) swap n for m

Thanks, Stevie Gee - didn't see that one. Now, left trying to puzzle the other one out!

Soften, cushion

S(pins), pins removed and
Often, over and over.

Many thanks, Malone - not too difficult, but it had me perplexed!

13d "Pet around house, note, runs in part of dash" (10)
???H???T?R

21a "Cats track mouse heartlessly by second track" (6)

M???R?

Any help much appreciated

21 Memory, Cats track, song from 'Cats' the musical. ME = mouse heartlessly, Mo, second and Ry, railway, tracks.

13 Tachometer, part of dash/dash board.

13...

Tac = Cat, pet, reversed
Home = house
Te = note (music)
R = runs.

Hi,
46d Very masculine ruler in ruin (7).
Looks like 'butcher' but can't see the 'ruler in ruin'.

50d Good health leaving queen's place (5).
P-s-t