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I think I have an incorrect answer thowing off the whole corner but here are the clues and what I have (bear in mind one or more of the letters might be off!)

2d Board a rail service E?T???N
3d Pompously Moralising S?N???T???S
4d Calculate R?C???
16a Duenna F???????O

Given I have a problem with 2-4d the first letters I have could be wrong. I have 'overstretched' as an answer to 'too extended'

Ta.

Entrain
Sententious
for the 1st two.

2 entrain

3 sanctimonious

4 reckon

sorry didnt count for 3 LOL

Calculate - Reckon?

Good start!

16a now F?A?T?O?O

sorry F?A?E?O?O

Answer should be chaperone - I think

actually the last O is wrong as triad is not terrorist. Grr!

F?A?T?O??

Got it! thanks for the help

16a is chaperone
20a ornate
24a discourse
1d overcrowd
5d threesome (oh err)